4,837 research outputs found

    Epitaxial strain effects in the spinel ferrites CoFe2O4 and NiFe2O4 from first principles

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    The inverse spinels CoFe2O4 and NiFe2O4, which have been of particular interest over the past few years as building blocks of artificial multiferroic heterostructures and as possible spin-filter materials, are investigated by means of density functional theory calculations. We address the effect of epitaxial strain on the magneto-crystalline anisotropy and show that, in agreement with experimental observations, tensile strain favors perpendicular anisotropy, whereas compressive strain favors in-plane orientation of the magnetization. Our calculated magnetostriction constants λ100\lambda_{100} of about -220 ppm for CoFe2O4 and -45 ppm for NiFe2O4 agree well with available experimental data. We analyze the effect of different cation arrangements used to represent the inverse spinel structure and show that both LSDA+U and GGA+U allow for a good quantitative description of these materials. Our results open the way for further computational investigations of spinel ferrites

    Signature of frustrated moments in quantum critical CePd1−x_{1-x}Nix_xAl

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    CePdAl with Ce 4f4f moments forming a distorted kagom\'e network is one of the scarce materials exhibiting Kondo physics and magnetic frustration simultaneously. As a result, antiferromagnetic (AF) order setting in at TN=2.7T_{\mathrm{N}} = 2.7~K encompasses only two thirds of the Ce moments. We report measurements of the specific heat, CC, and the magnetic Gr\"uneisen parameter, Γmag\Gamma_{\rm mag}, on single crystals of CePd1−x_{1-x}Nix_xAl with x≤0.16x\leq 0.16 at temperatures down to 0.05~K and magnetic fields BB up to 88~T. Field-induced quantum criticality for various concentrations is observed with the critical field decreasing to zero at xc≈0.15x_c\approx 0.15. Remarkably, two-dimensional (2D) AF quantum criticality of Hertz-Millis-Moriya type arises for x=0.05x=0.05 and x=0.1x=0.1 at the suppression of 3D magnetic order. Furthermore, Γmag(B)\Gamma_{\rm mag}(B) shows an additional contribution near 2.52.5~T for all concentrations which is ascribed to correlations of the frustrated one third of Ce moments.Comment: 5+2 pages with 4+3 figure

    Optical absorption of non-interacting tight-binding electrons in a Peierls-distorted chain at half band-filling

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    In this first of three articles on the optical absorption of electrons in half-filled Peierls-distorted chains we present analytical results for non-interacting tight-binding electrons. We carefully derive explicit expressions for the current operator, the dipole transition matrix elements, and the optical absorption for electrons with a cosine dispersion relation of band width WW and dimerization parameter δ\delta. New correction (``η\eta''-)terms to the current operator are identified. A broad band-to-band transition is found in the frequency range Wδ<ω<WW\delta < \omega < W whose shape is determined by the joint density of states for the upper and lower Peierls subbands and the strong momentum dependence of the transition matrix elements.Comment: 17 pages REVTEX 3.0, 2 postscript figures; hardcopy versions before May 96 are obsolete; accepted for publication in The Philosophical Magazine

    Magnetic and structural quantum phase transitions in CeCu6-xAux are independent

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    The heavy-fermion compound CeCu6−x_{6-x}Aux_x has become a model system for unconventional magnetic quantum criticality. For small Au concentrations 0≤x<0.160 \leq x < 0.16, the compound undergoes a structural transition from orthorhombic to monoclinic crystal symmetry at a temperature TsT_{s} with Ts→0T_{s} \rightarrow 0 for x≈0.15x \approx 0.15. Antiferromagnetic order sets in close to x≈0.1x \approx 0.1. To shed light on the interplay between quantum critical magnetic and structural fluctuations we performed neutron-scattering and thermodynamic measurements on samples with 0≤x≤0.30 \leq x\leq 0.3. The resulting phase diagram shows that the antiferromagnetic and monoclinic phase coexist in a tiny Au concentration range between x≈0.1x\approx 0.1 and 0.150.15. The application of hydrostatic and chemical pressure allows to clearly separate the transitions from each other and to explore a possible effect of the structural transition on the magnetic quantum critical behavior. Our measurements demonstrate that at low temperatures the unconventional quantum criticality exclusively arises from magnetic fluctuations and is not affected by the monoclinic distortion.Comment: 5 pages, 3 figure

    The long noncoding RNA neuroLNC regulates presynaptic activity by interacting with the neurodegeneration-associated protein TDP-43

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    The cellular and the molecular mechanisms by which long noncoding RNAs (lncRNAs) may regulate presynaptic function and neuronal activity are largely unexplored. Here, we established an integrated screening strategy to discover lncRNAs implicated in neurotransmitter and synaptic vesicle release. With this approach, we identified neuroLNC, a neuron-specific nuclear lncRNA conserved from rodents to humans. NeuroLNC is tuned by synaptic activity and influences several other essential aspects of neuronal development including calcium influx, neuritogenesis, and neuronal migration in vivo. We defined the molecular interactors of neuroLNC in detail using chromatin isolation by RNA purification, RNA interactome analysis, and protein mass spectrometry. We found that the effects of neuroLNC on synaptic vesicle release require interaction with the RNA-binding protein TDP-43 (TAR DNA binding protein-43) and the selective stabilization of mRNAs encoding for presynaptic proteins. These results provide the first proof of an lncRNA that orchestrates neuronal excitability by influencing presynaptic function
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